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By tuning the chemistry of this polymer anchor and sidechains, we investigate how physical and technical properties of polymeric interphases influence Li electrodeposit morphology. It is unearthed that an interplay between elasticity and diffusivity contributes to an optimum interphase thickness and that greater interfacial power augments elastic stresses at a metal electrode to prevent away from airplane deposition. These results are explained making use of linear stability analysis of electrodeposition
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