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The data presented here are related to the research paper entitled "Green Earth pigments dispersions water dynamics at the interfaces". The nuclear magnetic resonance (NMR) relaxometry data are provided for various aqueous Green Earth (GE) pigments dispersions with volume fraction spanning approximately from 0.1 to 0.5. For two of them (Cyprus GE and Bohemian GE), the NMR relaxation profiles from 10 kHz to 30 MHz (1H frequency) is given for several temperatures spanning from 293 to 318K. In addition, the X-ray diffraction pattern is provided for France GE (
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