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Controlling the interfacial effect is facing challenges because of the weak interactions between the inorganic and the organic materials. We found that the silane coupling agents with -NH2 groups (e.g., KH55 play a key role as a molecular bridge that links an inorganic silica template with an organic precursor (i.e., pyrrole) in the process of constructing a spherical silica core-polypyrrole shell structure. The molecular bridge is also suitable for inorganic core templates with cube or rod shapes for the construction of different core-
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