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Our approach of increasing the system's complexity to reduce the accessibility of neighboring structures should be generalizable to other systems beyond the self-assembly of tubules.Macroscopic conformation of individual graphene sheets serves as the backbone of translating their intrinsic merits towards multifunctional practical applications. However, controllable and continuous assemblies of graphene-based nanomaterials to create stable macroscopic structural components are always in face of great challenge. We have developed a scalab
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