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Hydrophobic solutes significantly alter the water hydrogen bond network. The local alteration of solvation structures gets reflected in the vibrational spectroscopic signal. Although it is possible to detect this microscopic feature by modern infrared spectroscopy, bulk phase spectra often come with a formidable challenge of establishing the connection of experimental spectra to molecular structures. Theoretical spectroscopy can serve as a more powerful tool where spectroscopic data cannot provide the microscopic picture. In the present
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