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In this paper, we determine the degree to which changes can be induced in the equilibrium thermal diffusivity and conductivity of a material via a selective nonequilibrium infrared stimulation mechanism for phonons. Using the molecular crystal RDX, we use detailed momentum-dependent coupling information across the entire Brillouin zone and the phonon gas model to show that stimulating selected modes in the spectrum of a target material can induce substantial changes in the overall thermal transport properties. Specifically in the case of
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