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Herein, a flexible ceramic/polymer HSE is prepared via in situ coupling effect. Ceramic and polymer tend to be closely combined by strong substance bonds, hence the issue of user interface compatibility is settled as well as the ions can transfer quickly by an expressway. The as-prepared membrane shows an ionic conductivity of 9.83 × 10-4 S cm-1 at room temperature and a high Li+ transference numbers of 0.68. This in situ coupling effect technique provides a good way to solve the issue o
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